A Novel Metastable Pentavalent Plutonium Solid Phase on the Pathway from Aqueous Plutonium(VI) to PuO(2) Nanoparticles

Here we provide evidence that the formation of PuO(2) nanoparticles from oxidized Pu(VI) under alkaline conditions proceeds through the formation of an intermediate Pu(V) solid phase, similar to NH(4)PuO(2)CO(3), which is stable over a period of several months. For the first time, state‐of‐the‐art e...

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Detalhes bibliográficos
Publicado no:Angew Chem Int Ed Engl
Main Authors: Kvashnina, Kristina O., Romanchuk, Anna Yu., Pidchenko, Ivan, Amidani, Lucia, Gerber, Evgeny, Trigub, Alexander, Rossberg, Andre, Weiss, Stephan, Popa, Karin, Walter, Olaf, Caciuffo, Roberto, Scheinost, Andreas C., Butorin, Sergei M., Kalmykov, Stepan N.
Formato: Artigo
Idioma:Inglês
Publicado em: John Wiley and Sons Inc. 2019
Assuntos:
Communications
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC6900038/
https://ncbi.nlm.nih.gov/pubmed/31621992
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/anie.201911637
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