Elucidation of near-resonance vibronic coherence lifetimes by nonadiabatic electronic-vibrational state character mixing

Recent work suggests that the long-lived coherences observed in both natural and artificial light-harvesting systems (such as the Fenna–Matthews–Olson complex) could be attributed to the mixing of the pigments’ electronic and vibrational degrees of freedom. To investigate the underlying mechanism of...

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Udgivet i:Proc Natl Acad Sci U S A
Main Authors: Yeh, Shu-Hao, Hoehn, Ross D., Allodi, Marco A., Engel, Gregory S., Kais, Sabre
Format: Artigo
Sprog:Inglês
Udgivet: National Academy of Sciences 2019
Fag:
Interfaces and Mixing: Nonequilibrium Transport Across the Scales Special Feature
Online adgang:https://ncbi.nlm.nih.gov/pmc/articles/PMC6744865/
https://ncbi.nlm.nih.gov/pubmed/30093387
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1073/pnas.1701390115
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