Llwytho...

Biocatalytic Carbon-Hydrogen and Carbon-Fluorine Bond Cleavage through Hydroxylation Promoted by a Histidyl-Ligated Heme Enzyme

LmbB2 is a peroxygenase-like enzyme that hydroxylates L-tyrosine to L-3,4-dihydroxyphenylalanine (DOPA) in the presence of hydrogen peroxide. However, its heme cofactor is ligated by a proximal histidine, not cysteine. We show that LmbB2 can oxidize L-tyrosine analogs with ring-deactivated substitue...

Disgrifiad llawn

Wedi'i Gadw mewn:
Manylion Llyfryddiaeth
Cyhoeddwyd yn:ACS Catal
Prif Awduron: Wang, Yifan, Davis, Ian, Shin, Inchul, Wherritt, Daniel J., Griffith, Wendell P., Dornevil, Kednerlin, Colabroy, Keri L., Liu, Aimin
Fformat: Artigo
Iaith:Inglês
Cyhoeddwyd: 2019
Pynciau:
Mynediad Ar-lein:https://ncbi.nlm.nih.gov/pmc/articles/PMC6660019/
https://ncbi.nlm.nih.gov/pubmed/31355048
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/acscatal.9b00231
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