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Acylation Reactions of Dibenzo‐7‐phosphanorbornadiene: DFT Mechanistic Insights

Extensive DFT calculations provide deep mechanistic insights into the acylation reactions of tert‐butyl dibenzo‐7‐phosphanobornadiene with PhCOX (X=Cl, Br, I, OTf) in CH(2)Cl(2) solution. Such reactions are initialized by the nucleophilic P⋅⋅⋅C attack to the carbonyl group to form the acylphosphoniu...

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Publicat a:ChemistryOpen
Autors principals: Qu, Zheng‐Wang, Zhu, Hui, Grimme, Stefan
Format: Artigo
Idioma:Inglês
Publicat: John Wiley and Sons Inc. 2019
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Accés en línia:https://ncbi.nlm.nih.gov/pmc/articles/PMC6594351/
https://ncbi.nlm.nih.gov/pubmed/31293872
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/open.201900176
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