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Accurate Probabilities for Highly Activated Reaction of Polyatomic Molecules on Surfaces Using a High-Dimensional Neural Network Potential: CHD(3) + Cu(111)

[Image: see text] An accurate description of reactive scattering of molecules on metal surfaces often requires the modeling of energy transfer between the molecule and the surface phonons. Although ab initio molecular dynamics (AIMD) can describe this energy transfer, AIMD is at present untractable...

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Publicat a:J Phys Chem Lett
Autors principals: Gerrits, N., Shakouri, Khosrow, Behler, Jörg, Kroes, Geert-Jan
Format: Artigo
Idioma:Inglês
Publicat: American Chemical Society 2019
Accés en línia:https://ncbi.nlm.nih.gov/pmc/articles/PMC6477808/
https://ncbi.nlm.nih.gov/pubmed/30922058
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/acs.jpclett.9b00560
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