Quantum electrodynamics at room temperature coupling a single vibrating molecule with a plasmonic nanocavity

Interactions between a single emitter and cavity provide the archetypical system for fundamental quantum electrodynamics. Here we show that a single molecule of Atto647 aligned using DNA origami interacts coherently with a sub-wavelength plasmonic nanocavity, approaching the cooperative regime even...

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Udgivet i:Nat Commun
Main Authors: Ojambati, Oluwafemi S., Chikkaraddy, Rohit, Deacon, William D., Horton, Matthew, Kos, Dean, Turek, Vladimir A., Keyser, Ulrich F., Baumberg, Jeremy J.
Format: Artigo
Sprog:Inglês
Udgivet: Nature Publishing Group UK 2019
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Article
Online adgang:https://ncbi.nlm.nih.gov/pmc/articles/PMC6400948/
https://ncbi.nlm.nih.gov/pubmed/30837456
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1038/s41467-019-08611-5
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