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Impact of nuclear quantum effects on the structural inhomogeneity of liquid water

The 2D Raman–terahertz (THz) response of liquid water is studied in dependence of temperature and isotope substitution ([Formula: see text] O, [Formula: see text] O, and [Formula: see text] O). In either case, a very short-lived (i.e., between 75 and 95 fs) echo is observed that reports on the inhom...

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Bibliografiske detaljer
Udgivet i:Proc Natl Acad Sci U S A
Main Authors: Berger, Arian, Ciardi, Gustavo, Sidler, David, Hamm, Peter, Shalit, Andrey
Format: Artigo
Sprog:Inglês
Udgivet: National Academy of Sciences 2019
Fag:
Online adgang:https://ncbi.nlm.nih.gov/pmc/articles/PMC6377483/
https://ncbi.nlm.nih.gov/pubmed/30692247
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1073/pnas.1818182116
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