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Enantioselective Lewis Acid Catalyzed ortho Photocycloaddition of Olefins to Phenanthrene‐9‐carboxaldehydes

Visible‐light irradiation (λ=457 nm) enabled the enantioselective ortho photocycloaddition of olefins to phenanthrene‐9‐carboxaldehydes (15 examples, 46–93 % yield, 82–98 % ee). A chiral oxazaborolidine Lewis acid (20 mol %) was employed as the catalyst. It operates by coordination to the aldehyde i...

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Detalhes bibliográficos
Publicado no:Angew Chem Int Ed Engl
Main Authors: Stegbauer, Simone, Jandl, Christian, Bach, Thorsten
Formato: Artigo
Idioma:Inglês
Publicado em: John Wiley and Sons Inc. 2018
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC6220838/
https://ncbi.nlm.nih.gov/pubmed/30225921
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/anie.201808919
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