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On the origin of the elusive first intermediate of CO(2) electroreduction
We resolve the long-standing controversy about the first step of the CO(2) electroreduction to fuels in aqueous electrolytes by providing direct spectroscopic evidence that the first intermediate of the CO(2) conversion to formate on copper is a carboxylate anion *CO(2)(−) coordinated to the surface...
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| Publicado no: | Proc Natl Acad Sci U S A |
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| Main Authors: | , , |
| Formato: | Artigo |
| Idioma: | Inglês |
| Publicado em: |
National Academy of Sciences
2018
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| Assuntos: | |
| Acesso em linha: | https://ncbi.nlm.nih.gov/pmc/articles/PMC6176638/ https://ncbi.nlm.nih.gov/pubmed/30224482 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1073/pnas.1802256115 |
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