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Machine Learning Adaptive Basis Sets for Efficient Large Scale Density Functional Theory Simulation

[Image: see text] It is chemically intuitive that an optimal atom centered basis set must adapt to its atomic environment, for example by polarizing toward nearby atoms. Adaptive basis sets of small size can be significantly more accurate than traditional atom centered basis sets of the same size. T...

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Foilsithe in:J Chem Theory Comput
Main Authors: Schütt, Ole, VandeVondele, Joost
Formáid: Artigo
Teanga:Inglês
Foilsithe: American Chemical Society 2018
Rochtain Ar Líne:https://ncbi.nlm.nih.gov/pmc/articles/PMC6096449/
https://ncbi.nlm.nih.gov/pubmed/29957943
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/acs.jctc.8b00378
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