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Catalytic iron-carbene intermediate revealed in a cytochrome c carbene transferase

Recently, heme proteins have been discovered and engineered by directed evolution to catalyze chemical transformations that are biochemically unprecedented. Many of these nonnatural enzyme-catalyzed reactions are assumed to proceed through a catalytic iron porphyrin carbene (IPC) intermediate, altho...

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Pubblicato in:Proc Natl Acad Sci U S A
Autori principali: Lewis, Russell D., Garcia-Borràs, Marc, Chalkley, Matthew J., Buller, Andrew R., Houk, K. N., Kan, S. B. Jennifer, Arnold, Frances H.
Natura: Artigo
Lingua:Inglês
Pubblicazione: National Academy of Sciences 2018
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Accesso online:https://ncbi.nlm.nih.gov/pmc/articles/PMC6048479/
https://ncbi.nlm.nih.gov/pubmed/29946033
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1073/pnas.1807027115
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