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Time-dependent view of an isotope effect in electron-nuclear nonequilibrium dynamics with applications to N(2)

Isotopic fractionation in the photodissociation of N(2) could explain the considerable variation in the (14)N/(15)N ratio in different regions of our galaxy. We previously proposed that such an isotope effect is due to coupling of photoexcited bound valence and Rydberg electronic states in the frequ...

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Detalles Bibliográficos
Publicado en:Proc Natl Acad Sci U S A
Main Authors: Ajay, Jayanth S., Komarova, Ksenia G., Remacle, Francoise, Levine, R. D.
Formato: Artigo
Idioma:Inglês
Publicado: National Academy of Sciences 2018
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Acceso en liña:https://ncbi.nlm.nih.gov/pmc/articles/PMC6003327/
https://ncbi.nlm.nih.gov/pubmed/29784776
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1073/pnas.1804455115
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