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Assembly of the Limonoid Architecture by a Divergent Approach: Total Synthesis of (±)-Andirolide N via (±)-8α-Hydroxycarapin

We report the first total synthesis of the limonoid andirolide N using a 12-step sequence from commercially available materials. The final step of this route demonstrates the chemical feasibility of our biosynthetic proposal that andirolide N arises from 8α-hydroxycarapin. The strategic use of a deg...

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Detalhes bibliográficos
Publicado no:J Am Chem Soc
Main Authors: Schuppe, Alexander W., Newhouse, Timothy R.
Formato: Artigo
Idioma:Inglês
Publicado em: 2017
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC5928519/
https://ncbi.nlm.nih.gov/pubmed/28001380
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.6b12268
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