Intramolecular hydrogen-bonding in a cobalt aqua complex and electrochemical water oxidation activity

Water oxidation is catalysed in Nature by a redox cofactor embedded in a hydrogen-bonded network designed to orchestrate proton transfer throughout the challenging 4 electron reaction. In order to mimic aspects of this microenvironment, [CoL(DMA)(CH(3)CN)(2)][BF(4)](2) (2) was synthesized, where L(D...

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Udgivet i:Chem Sci
Main Authors: Khosrowabadi Kotyk, Juliet F., Hanna, Caitlin M., Combs, Rebecca L., Ziller, Joseph W., Yang, Jenny Y.
Format: Artigo
Sprog:Inglês
Udgivet: Royal Society of Chemistry 2018
Fag:
Chemistry
Online adgang:https://ncbi.nlm.nih.gov/pmc/articles/PMC5912104/
https://ncbi.nlm.nih.gov/pubmed/29732059
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1039/c7sc04960a
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