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Gold-catalyzed Fluorination of Alkynyl Esters and Ketones: Efficient Access to Fluorinated 1,3-Dicarbonyl Compounds

We developed an efficient synthesis of 2-fluoro-1,3-dicarbonyl compounds using readily available alkynyl ketones or esters as starting material. The key step is the insertion of hydrogen fluoride (HF) to the gold carbene intermediate generated from cationic gold catalyzed addition of N-oxides to alk...

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Detalhes bibliográficos
Publicado no:Adv Synth Catal
Main Authors: Zeng, Xiaojun, Lu, Zhichao, Liu, Shiwen, Hammond, Gerald B., Xu, Bo
Formato: Artigo
Idioma:Inglês
Publicado em: 2017
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC5824727/
https://ncbi.nlm.nih.gov/pubmed/29483850
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/adsc.201701179
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