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Enantioselective Total Synthesis of Cannogenol-3-O-α-L-Rhamnoside via Sequential Cu(II)-Catalyzed Michael Addition/Intramolecular Aldol Cyclization Reactions

A concise and scalable enantioselective total synthesis of the natural cardenolides cannogenol and cannogenol-3-O-α-L-rhamnoside has been achieved in 19 linear steps. The synthesis features a Cu(II)-catalyzed enantioselective and diastereoselective Michael reaction/tandem aldol cyclization and a one...

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Vydáno v:Org Lett
Hlavní autoři: Bhattarai, Bijay, Nagorny, Pavel
Médium: Artigo
Jazyk:Inglês
Vydáno: 2017
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On-line přístup:https://ncbi.nlm.nih.gov/pmc/articles/PMC5768146/
https://ncbi.nlm.nih.gov/pubmed/29244520
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/acs.orglett.7b03513
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