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Slow Cooling of Hot Polarons in Halide Perovskite Solar Cells

[Image: see text] Halide perovskites show unusual thermalization kinetics for above-bandgap photoexcitation. We explain this as a consequence of excess energy being deposited into discrete large polaron states. The crossover between low-fluence and high-fluence “phonon bottleneck” cooling is due to...

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Veröffentlicht in:ACS Energy Lett
Hauptverfasser: Frost, Jarvist Moore, Whalley, Lucy D., Walsh, Aron
Format: Artigo
Sprache:Inglês
Veröffentlicht: American Chemical Society 2017
Online Zugang:https://ncbi.nlm.nih.gov/pmc/articles/PMC5727468/
https://ncbi.nlm.nih.gov/pubmed/29250603
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/acsenergylett.7b00862
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