Bioinspired design of redox-active ligands for multielectron catalysis: effects of positioning pyrazine reservoirs on cobalt for electro- and photocatalytic generation of hydrogen from water

Mononuclear metalloenzymes in nature can function in cooperation with precisely positioned redox-active organic cofactors in order to carry out multielectron catalysis. Inspired by the finely tuned redox management of these bioinorganic systems, we present the design, synthesis, and experimental and...

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Bibliografiske detaljer
Udgivet i:Chem Sci
Main Authors: Jurss, Jonah W., Khnayzer, Rony S., Panetier, Julien A., El Roz, Karim A., Nichols, Eva M., Head-Gordon, Martin, Long, Jeffrey R., Castellano, Felix N., Chang, Christopher J.
Format: Artigo
Sprog:Inglês
Udgivet: Royal Society of Chemistry 2015
Fag:
Chemistry
Online adgang:https://ncbi.nlm.nih.gov/pmc/articles/PMC5664355/
https://ncbi.nlm.nih.gov/pubmed/29142725
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1039/c5sc01414j
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