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Catalytic Allylic Oxidation of Cyclic Enamides and 3,4-Dihydro-2H-Pyrans by TBHP

Allylic oxidation of heteroatom substituted cyclic alkenes by tert-butyl hydroperoxide (70% TBHP in water) using catalytic dirhodium caprolactamate [Rh(2)(cap)(4)] forms enone products with a variety of 2-substituted cyclic enamides and 3,4-dihyro-2H-pyrans. These reactions occur under mild reaction...

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Detalhes bibliográficos
Publicado no:J Org Chem
Main Authors: Yu, Yang, Humeidi, Ranad, Alleyn, James R., Doyle, Michael P.
Formato: Artigo
Idioma:Inglês
Publicado em: 2017
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC5660929/
https://ncbi.nlm.nih.gov/pubmed/28723085
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/acs.joc.7b01163
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