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Carbon nitride–TiO(2) hybrid modified with hydrogenase for visible light driven hydrogen production

A system consisting of a [NiFeSe]–hydrogenase (H(2)ase) grafted on the surface of a TiO(2) nanoparticle modified with polyheptazine carbon nitride polymer, melon (CN(x)) is reported. This semi-biological assembly shows a turnover number (TON) of more than 5.8 × 10(5) mol H(2) (mol H(2)ase)(–1) after...

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Publicado en:Chem Sci
Main Authors: Caputo, Christine A., Wang, Lidong, Beranek, Radim, Reisner, Erwin
Formato: Artigo
Idioma:Inglês
Publicado: Royal Society of Chemistry 2015
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Acceso en liña:https://ncbi.nlm.nih.gov/pmc/articles/PMC5512016/
https://ncbi.nlm.nih.gov/pubmed/28757952
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1039/c5sc02017d
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