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Mechanism of photocatalytic water oxidation on small TiO(2) nanoparticles

We present the first unconstrained nonadiabatic molecular dynamics (NAMD) simulations of photocatalytic water oxidation by small hydrated TiO(2) nanoparticles using Tully surface hopping and time-dependent density functional theory. The results indicate that ultrafast electron–proton transfer from p...

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Detalhes bibliográficos
Publicado no:Chem Sci
Main Authors: Muuronen, Mikko, Parker, Shane M., Berardo, Enrico, Le, Alexander, Zwijnenburg, Martijn A., Furche, Filipp
Formato: Artigo
Idioma:Inglês
Publicado em: Royal Society of Chemistry 2017
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC5407260/
https://ncbi.nlm.nih.gov/pubmed/28507672
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1039/c6sc04378j
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