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Photochemical pump and NMR probe to monitor the formation and kinetics of hyperpolarized metal dihydrides

On reaction of IrI(CO)(PPh(3))(2) 1 with para-hydrogen (p-H(2)), Ir(H)(2)I(CO)(PPh(3))(2) 2 is formed which exhibits strongly enhanced (1)H NMR signals for its hydride resonances. Complex 2 also shows similar enhancement of its NMR spectra when it is irradiated under p-H(2). We report the use of thi...

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Detalhes bibliográficos
Publicado no:Chem Sci
Main Authors: Procacci, Barbara, Aguiar, Pedro M., Halse, Meghan E., Perutz, Robin N., Duckett, Simon B.
Formato: Artigo
Idioma:Inglês
Publicado em: Royal Society of Chemistry 2016
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC5363785/
https://ncbi.nlm.nih.gov/pubmed/28451144
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1039/c6sc01956k
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