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Inner-sphere vs. outer-sphere reduction of uranyl supported by a redox-active, donor-expanded dipyrrin
The uranyl(vi) complex UO(2)Cl(L) of the redox-active, acyclic diimino-dipyrrin anion, L(–) is reported and its reaction with inner- and outer-sphere reductants studied. Voltammetric, EPR-spectroscopic and X-ray crystallographic studies show that chemical reduction by the outer-sphere reagent CoCp(2...
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| Publicado en: | Chem Sci |
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| Autores principales: | , , , , , , , , , |
| Formato: | Artigo |
| Lenguaje: | Inglês |
| Publicado: |
Royal Society of Chemistry
2017
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| Materias: | |
| Acceso en línea: | https://ncbi.nlm.nih.gov/pmc/articles/PMC5304617/ https://ncbi.nlm.nih.gov/pubmed/28451154 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1039/c6sc02912d |
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