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Electrocatalytic and Solar‐Driven CO(2) Reduction to CO with a Molecular Manganese Catalyst Immobilized on Mesoporous TiO(2)

Electrocatalytic CO(2) reduction to CO was achieved with a novel Mn complex, fac‐[MnBr(4,4′‐bis(phosphonic acid)‐2,2′‐bipyridine)(CO)(3)] (MnP), immobilized on a mesoporous TiO(2) electrode. A benchmark turnover number of 112±17 was attained with these TiO(2)|MnP electrodes after 2 h electrolysis. P...

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Veröffentlicht in:Angew Chem Int Ed Engl
Hauptverfasser: Rosser, Timothy E., Windle, Christopher D., Reisner, Erwin
Format: Artigo
Sprache:Inglês
Veröffentlicht: John Wiley and Sons Inc. 2016
Schlagworte:
Online Zugang:https://ncbi.nlm.nih.gov/pmc/articles/PMC5074277/
https://ncbi.nlm.nih.gov/pubmed/27110904
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/anie.201601038
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