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Enantioselective Rhodium-Catalyzed Isomerization of 4-Iminocrotonates: Asymmetric Synthesis of a Unique Chiral Synthon

An enantioselective isomerization of 4-iminocrotonates catalyzed by a rhodium(I)/phosphoramidite complex is described. This reaction uses widely available amines to couple with 4-oxocrotonate to provide a convenient access to a central chiral building block in good yield and high enantioselectivity....

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Pubblicato in:J Am Chem Soc
Autori principali: Zhang, Wen-Zhen, Chu, John C. K., Oberg, Kevin M., Rovis, Tomislav
Natura: Artigo
Lingua:Inglês
Pubblicazione: 2015
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Accesso online:https://ncbi.nlm.nih.gov/pmc/articles/PMC4986700/
https://ncbi.nlm.nih.gov/pubmed/25580807
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ja510348p
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