Nitrogenase-mimic iron-containing chalcogels for photochemical reduction of dinitrogen to ammonia

A nitrogenase-inspired biomimetic chalcogel system comprising double-cubane [Mo(2)Fe(6)S(8)(SPh)(3)] and single-cubane (Fe(4)S(4)) biomimetic clusters demonstrates photocatalytic N(2) fixation and conversion to NH(3) in ambient temperature and pressure conditions. Replacing the Fe(4)S(4) clusters in...

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Detalhes bibliográficos
Publicado no:Proc Natl Acad Sci U S A
Main Authors: Liu, Jian, Kelley, Matthew S., Wu, Weiqiang, Banerjee, Abhishek, Douvalis, Alexios P., Wu, Jinsong, Zhang, Yongbo, Schatz, George C., Kanatzidis, Mercouri G.
Formato: Artigo
Idioma:Inglês
Publicado em: National Academy of Sciences 2016
Assuntos:
Physical Sciences
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC4878479/
https://ncbi.nlm.nih.gov/pubmed/27140630
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1073/pnas.1605512113
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