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Active sites and mechanisms for H(2)O(2) decomposition over Pd catalysts

A combination of periodic, self-consistent density functional theory (DFT-GGA-PW91) calculations, reaction kinetics experiments on a SiO(2)-supported Pd catalyst, and mean-field microkinetic modeling are used to probe key aspects of H(2)O(2) decomposition on Pd in the absence of cofeeding H(2). We c...

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Detalhes bibliográficos
Publicado no:Proc Natl Acad Sci U S A
Main Authors: Plauck, Anthony, Stangland, Eric E., Dumesic, James A., Mavrikakis, Manos
Formato: Artigo
Idioma:Inglês
Publicado em: National Academy of Sciences 2016
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC4833276/
https://ncbi.nlm.nih.gov/pubmed/27006504
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1073/pnas.1602172113
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