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A Visible Light-Mediated Radical Smiles Rearrangement and its Application to the Synthesis of a Difluorospirocyclic ORL-1 Antagonist()

A visible light-mediated radical Smiles rearrangement has been developed to address the challenging synthesis of a gem-difluoro group present in an opioid receptor-like 1 (ORL-1) antagonist currently in development. This method led to the direct and efficient introduction of the difluoroethanol moti...

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Detalhes bibliográficos
Publicado no:Angew Chem Int Ed Engl
Main Authors: Douglas, James J., Albright, Haley, Sevrin, Martin J., Cole, Kevin P., Stephenson, Corey R. J.
Formato: Artigo
Idioma:Inglês
Publicado em: 2015
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC4725294/
https://ncbi.nlm.nih.gov/pubmed/26474077
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/anie.201507369
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