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Ideal probe single-molecule experiments reveal the intrinsic dynamic heterogeneity of a supercooled liquid

The concept of dynamic heterogeneity and the picture of the supercooled liquid as a mosaic of environments with distinct dynamics that interchange in time have been invoked to explain the nonexponential relaxations measured in these systems. The spatial extent and temporal persistence of these regio...

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Pubblicato in:Proc Natl Acad Sci U S A
Autori principali: Paeng, Keewook, Park, Heungman, Hoang, Dat Tien, Kaufman, Laura J.
Natura: Artigo
Lingua:Inglês
Pubblicazione: National Academy of Sciences 2015
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Accesso online:https://ncbi.nlm.nih.gov/pmc/articles/PMC4413315/
https://ncbi.nlm.nih.gov/pubmed/25825739
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1073/pnas.1424636112
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