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Base-enhanced catalytic water oxidation by a carboxylate–bipyridine Ru(II) complex
In aqueous solution above pH 2.4 with 4% (vol/vol) CH(3)CN, the complex [Ru(II)(bda)(isoq)(2)] (bda is 2,2′-bipyridine-6,6′-dicarboxylate; isoq is isoquinoline) exists as the open-arm chelate, [Ru(II)(CO(2)-bpy-CO(2)(−))(isoq)(2)(NCCH(3))], as shown by (1)H and (13)C-NMR, X-ray crystallography, and...
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| 出版年: | Proc Natl Acad Sci U S A |
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| 主要な著者: | , , , , , , , |
| フォーマット: | Artigo |
| 言語: | Inglês |
| 出版事項: |
National Academy of Sciences
2015
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| 主題: | |
| オンライン･アクセス: | https://ncbi.nlm.nih.gov/pmc/articles/PMC4413278/ https://ncbi.nlm.nih.gov/pubmed/25848035 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1073/pnas.1500245112 |
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