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Radiationless relaxation in “large” molecules: Experimental evidence for preparation of true molecular eigenstates and Born-Oppenheimer states by a coherent light source

Photon absorption and emission by molecules that undergo radiationless transitions are examined using the single modes of lasers having well-defined coherence properties. Contrary to the usual beliefs, where it is assumed that the molecule is prepared in a Born-Oppenheimer singlet state and then “cr...

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Detalhes bibliográficos
Publicado no:Proc Natl Acad Sci U S A
Principais autores: Zewail, A. H., Orlowski, T. E., Jones, K. E.
Formato: Artigo
Idioma:Inglês
Publicado em: National Academy of Sciences 1977
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.govhttps://pmc.ncbi.nlm.nih.gov/articles/PMC430735/
https://ncbi.nlm.nih.govhttps://pubmed.ncbi.nlm.nih.gov/16578747/
https://ncbi.nlm.nih.govhttps://doi.org/10.1073/pnas.74.4.1310
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