Anomalously large isotope effect in the glass transition of water

We present the discovery of an unusually large isotope effect in the structural relaxation and the glass transition temperature T(g) of water. Dielectric relaxation spectroscopy of low-density as well as of vapor-deposited amorphous water reveal T(g) differences of 10 ± 2 K between H(2)O and D(2)O,...

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Detalhes bibliográficos
Publicado no:Proc Natl Acad Sci U S A
Main Authors: Gainaru, Catalin, Agapov, Alexander L., Fuentes-Landete, Violeta, Amann-Winkel, Katrin, Nelson, Helge, Köster, Karsten W., Kolesnikov, Alexander I., Novikov, Vladimir N., Richert, Ranko, Böhmer, Roland, Loerting, Thomas, Sokolov, Alexei P.
Formato: Artigo
Idioma:Inglês
Publicado em: National Academy of Sciences 2014
Assuntos:
Physical Sciences
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC4267340/
https://ncbi.nlm.nih.gov/pubmed/25422420
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1073/pnas.1411620111
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