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Distance dependent charge separation and recombination in semiconductor/molecular catalyst systems for water splitting

The photoinduced reduction of three Co electrocatalysts immobilised on TiO(2) is 10(4) times faster than the reverse charge recombination. Both processes show an exponential dependence on the distance between the semiconductor and the catalytic core.

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Autors principals: Reynal, Anna, Willkomm, Janina, Muresan, Nicoleta M., Lakadamyali, Fezile, Planells, Miquel, Reisner, Erwin, Durrant, James R.
Format: Artigo
Idioma:Inglês
Publicat: Royal Society of Chemistry 2014
Matèries:
Accés en línia:https://ncbi.nlm.nih.gov/pmc/articles/PMC4183993/
https://ncbi.nlm.nih.gov/pubmed/25207748
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1039/c4cc05143b
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