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Distinguishing Electronic and Vibronic Coherence in 2D Spectra by Their Temperature Dependence

[Image: see text] Long-lived oscillations in 2D spectra of chlorophylls are at the heart of an ongoing debate. Their physical origin is either a multipigment effect, such as excitonic coherence, or localized vibrations. We show how relative phase differences of diagonal- and cross-peak oscillations...

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Main Authors: Perlík, Václav, Lincoln, Craig, Šanda, František, Hauer, Jürgen
Formato: Artigo
Idioma:Inglês
Publicado: American Chemical Society 2014
Acceso en liña:https://ncbi.nlm.nih.gov/pmc/articles/PMC3917822/
https://ncbi.nlm.nih.gov/pubmed/24527180
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jz402468c
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