Experimental and Computational X-ray Emission Spectroscopy as a Direct Probe of Protonation States in Oxo-Bridged Mn(IV)- Dimers Relevant to Redox-active Metalloproteins

The protonation state of oxo-bridges in nature is of profound importance for a variety of enzymes, including the Mn(4)CaO(5) cluster of Photosystem II and the Mn(2)O(2) cluster in Mn catalase. A set of dinuclear bis-μ-oxo-bridged Mn(IV) complexes in different protonation states was studied by Kβ emi...

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Main Authors: Lassalle-Kaiser, Benedikt, Boron, Thaddeus T., Krewald, Vera, Kern, Jan, Beckwith, Martha A., Schroeder, Henning, Alonso-Mori, Roberto, Nordlund, Dennis, Weng, Tsu-Chien, Sokaras, Dimosthenis, Neese, Frank, Bergmann, Uwe, Yachandra, Vittal K., DeBeer, Serena, Pecoraro, Vincent L., Yano, Junko
Formato: Artigo
Idioma:Inglês
Publicado em: 2013
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Article
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC3867288/
https://ncbi.nlm.nih.gov/pubmed/24161081
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ic400821g
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