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Enantioselective Synthesis of Angularly Substituted 1-Azabicylic Rings: Coupled Dynamic Kinetic Epimerization and Chirality Transfer

[Image: see text] A new strategy for enantioselective synthesis of azacyclic molecules in which dynamic kinetic equilibration of diastereomeric iminium ions precedes a stereochemistry-determining sigmatropic rearrangement is reported. The method is illustrated by the synthesis in high enantiomeric p...

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Detalhes bibliográficos
Main Authors: Aron, Zachary D., Ito, Tatsuya, May, Tricia L., Overman, Larry E., Wang, Jocelyn
Formato: Artigo
Idioma:Inglês
Publicado em: 2013
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC3843940/
https://ncbi.nlm.nih.gov/pubmed/24090405
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jo4018099
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