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Entangled Valence Electron-Hole Dynamics Revealed by Stimulated Attosecond X-ray Raman Scattering

We show that broadband x-ray pulses can create wavepackets of valence electrons and holes localized in the vicinity of a selected atom (nitrogen, oxygen or sulfur in cysteine) by stimulated resonant Raman scattering. The subsequent dynamics reveals highly correlated motions of entangled electrons an...

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Main Authors: Healion, Daniel, Zhang, Yu, Biggs, Jason D., Govind, Niranjan, Mukamel, Shaul
Format: Artigo
Jezik:Inglês
Izdano: 2012
Teme:
Online dostop:https://ncbi.nlm.nih.gov/pmc/articles/PMC3675902/
https://ncbi.nlm.nih.gov/pubmed/23755318
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jz300981w
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