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Mapping Enzymatic Catalysis Using the Effective Fragment Molecular Orbital Method: Towards all ab initio Biochemistry

We extend the Effective Fragment Molecular Orbital (EFMO) method to the frozen domain approach where only the geometry of an active part is optimized, while the many-body polarization effects are considered for the whole system. The new approach efficiently mapped out the entire reaction path of cho...

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Detalhes bibliográficos
Main Authors: Steinmann, Casper, Fedorov, Dmitri G., Jensen, Jan H.
Formato: Artigo
Idioma:Inglês
Publicado em: Public Library of Science 2013
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC3625203/
https://ncbi.nlm.nih.gov/pubmed/23593259
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1371/journal.pone.0060602
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