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Ultrafast photodriven intramolecular electron transfer from an iridium-based water-oxidation catalyst to perylene diimide derivatives

Photodriving the activity of water-oxidation catalysts is a critical step toward generating fuel from sunlight. The design of a system with optimal energetics and kinetics requires a mechanistic understanding of the single-electron transfer events in catalyst activation. To this end, we report here...

תיאור מלא

שמור ב:
מידע ביבליוגרפי
Main Authors: Vagnini, Michael T., Smeigh, Amanda L., Blakemore, James D., Eaton, Samuel W., Schley, Nathan D., D’Souza, Francis, Crabtree, Robert H., Brudvig, Gary W., Co, Dick T., Wasielewski, Michael R.
פורמט: Artigo
שפה:Inglês
יצא לאור: National Academy of Sciences 2012
נושאים:
גישה מקוונת:https://ncbi.nlm.nih.gov/pmc/articles/PMC3465409/
https://ncbi.nlm.nih.gov/pubmed/22586073
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1073/pnas.1202075109
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