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Anti-Arrhenius cleavage of covalent bonds in bottlebrush macromolecules on substrate

Spontaneous degradation of bottlebrush macromolecules on aqueous substrates was monitored by atomic force microscopy. Scission of C─C covalent bonds in the brush backbone occurred due to steric repulsion between the adsorbed side chains, which generated bond tension on the order of several nano-Newt...

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Bibliografiske detaljer
Main Authors: Lebedeva, Natalia V., Nese, Alper, Sun, Frank C., Matyjaszewski, Krzysztof, Sheiko, Sergei S.
Format: Artigo
Sprog:Inglês
Udgivet: National Academy of Sciences 2012
Fag:
Online adgang:https://ncbi.nlm.nih.gov/pmc/articles/PMC3386079/
https://ncbi.nlm.nih.gov/pubmed/22645366
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1073/pnas.1118517109
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