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A Single Site mutation (F429H) Converts the Enzyme CYP 2B4 into a Heme Oxygenase: A QM/MM Study

The intriguing deactivation of the cytochrome P450 (CYP) 2B4 enzyme induced by a mutation of a single residue, Phe429 to His, is explored by means of quantum mechanical/molecular mechanical (QM/MM) calculations of the O-OH bond activation of the (Fe(3+)OOH)(−) intermediate. It is found that the F429...

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Main Authors: Usharani, Dandamudi, Zazza, Costantino, Lai, Wenzhen, Chourasia, Mukesh, Waskell, Lucy, Shaik, Sason
格式: Artigo
語言:Inglês
出版: 2012
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在線閱讀:https://ncbi.nlm.nih.gov/pmc/articles/PMC3326604/
https://ncbi.nlm.nih.gov/pubmed/22356576
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ja211905e
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