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Ultrafast large-amplitude relocation of electronic charge in ionic crystals

The interplay of vibrational motion and electronic charge relocation in an ionic hydrogen-bonded crystal is mapped by X-ray powder diffraction with a 100 fs time resolution. Photoexcitation of the prototype material KH(2)PO(4) induces coherent low-frequency motions of the PO(4) tetrahedra in the ele...

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Main Authors: Zamponi, Flavio, Rothhardt, Philip, Stingl, Johannes, Woerner, Michael, Elsaesser, Thomas
格式: Artigo
語言:Inglês
出版: National Academy of Sciences 2012
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在線閱讀:https://ncbi.nlm.nih.gov/pmc/articles/PMC3325693/
https://ncbi.nlm.nih.gov/pubmed/22431621
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1073/pnas.1108206109
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