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Thionium Ion-initiated Medium-sized Ring Formation: The Total Synthesis of Asteriscunolide D
The first synthesis of the biologically active humulene natural product asteriscunolide D has been accomplished in nine steps without the use of protecting groups. The challenging 11-membered ring was forged via a diastereoselective thionium ion-initiated cyclization, which constitutes a formal aldo...
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| Main Authors: | , , , , |
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| Formato: | Artigo |
| Idioma: | Inglês |
| Publicado em: |
2012
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| Assuntos: | |
| Acesso em linha: | https://ncbi.nlm.nih.gov/pmc/articles/PMC3268366/ https://ncbi.nlm.nih.gov/pubmed/22236456 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ja210986f |
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