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Developing a Diastereoselective Intramolecular [4 + 3] Cycloaddition of Nitrogen-Stabilized Oxyallyl Cations Derived from N-Sulfonyl-Substituted Allenamides

[Image: see text] Efforts toward achieving a practical and diastereoselective intramolecular [4 + 3] cycloaddition of nitrogen-stabilized oxyallyl cations with tethered dienes are described. Epoxidation of N-sulfonyl substituted allenamides with dimethyldioxirane (DMDO) generates nitrogen-stabilized...

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Detalhes bibliográficos
Main Authors: Lohse, Andrew G., Hsung, Richard P., Leider, Mitchell D., Ghosh, Sunil K.
Formato: Artigo
Idioma:Inglês
Publicado em: 2011
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC3095656/
https://ncbi.nlm.nih.gov/pubmed/21449577
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jo200147h
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