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Evidence That Epoxide-Opening Cascades Promoted by Water Are Stepwise and Become Faster and More Selective After the First Cyclization

A detailed kinetic study of the endo-selective epoxide-opening cascade reaction of a diepoxy alcohol in neutral water was undertaken using (1)H NMR spectroscopy. The observation of monoepoxide intermediates resulting from initial endo and exo cyclization indicated that the cascade proceeds via a ste...

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Autori principali: Morten, Christopher J., Byers, Jeffery A., Jamison, Timothy F.
Natura: Artigo
Lingua:Inglês
Pubblicazione: 2011
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Accesso online:https://ncbi.nlm.nih.gov/pmc/articles/PMC3084897/
https://ncbi.nlm.nih.gov/pubmed/21235230
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ja1088748
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