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Extracting the Excitonic Hamiltonian of the Fenna-Matthews-Olson Complex Using Three-Dimensional Third-Order Electronic Spectroscopy

We extend traditional two-dimensional (2D) electronic spectroscopy into a third Fourier dimension without the use of additional optical interactions. By acquiring a set of 2D spectra evenly spaced in waiting time and dividing the area of the spectra into voxels, we can eliminate population dynamics...

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Détails bibliographiques
Auteurs principaux: Hayes, Dugan, Engel, Gregory S.
Format: Artigo
Langue:Inglês
Publié: The Biophysical Society 2011
Sujets:
Accès en ligne:https://ncbi.nlm.nih.gov/pmc/articles/PMC3077693/
https://ncbi.nlm.nih.gov/pubmed/21504741
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1016/j.bpj.2010.12.3747
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