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A(1),(3)-strain enabled retention of chirality during bis-cyclization of β-ketoamides: total synthesis of (−)-salinosporamide A and (−)-homosalinosporamide A

A concise, enantioselective synthesis of the Phase I anticancer agent, (−)-salinosporamide A, is described. The brevity of the described strategy stems from a key bis-cyclization of a β-keto tertiary amide, accomplished on gram scale, which retains optical purity enabled by A(1),(3)-strain rendering...

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Detalhes bibliográficos
Main Authors: Nguyen, Henry, Ma, Gil, Romo, Daniel
Formato: Artigo
Idioma:Inglês
Publicado em: 2010
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC2981177/
https://ncbi.nlm.nih.gov/pubmed/20498903
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1039/c0cc00607f
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