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Diastereoselective Nickel-Catalyzed Reductive Couplings of Aminoaldehydes and Alkynylsilanes: Application to the Synthesis of D-erythro-Sphingosine

[Image: see text] A strategy for the nickel-catalyzed reductive coupling of α-aminoaldehydes with silyl alkynes has been developed. The process proceeds with exceptional regiocontrol and diastereoselectivity. A variety of protected serinal derivatives were examined, and Garner aldehyde afforded the...

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Hlavní autoři: Sa-ei, Kanicha, Montgomery, John
Médium: Artigo
Jazyk:Inglês
Vydáno: 2009
Témata:
On-line přístup:https://ncbi.nlm.nih.gov/pmc/articles/PMC2902792/
https://ncbi.nlm.nih.gov/pubmed/20640041
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1016/j.tet.2009.05.029
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