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Generalized Kramers-Heisenberg expressions for stimulated Raman scattering and two-photon absorption

The frequency-domain pump-probe signal of a material system interacting with two quantum modes of the radiation field is recast in terms of products of scattering amplitudes (T matrix elements) rather than the third-order susceptibility Im χ((3)). The resulting expression offers a more intuitive phy...

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Detalhes bibliográficos
Main Authors: Roslyak, Oleksiy, Marx, Christoph A., Mukamel, Shaul
Formato: Artigo
Idioma:Inglês
Publicado em: 2009
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC2897726/
https://ncbi.nlm.nih.gov/pubmed/20613889
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1103/PhysRevA.79.063827
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