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Mode selectivity with polarization shaping in the mid-IR

We report that polarization-shaped mid-infrared (IR) pulses can be used to enhance the vibrational population of one mode over another in a coupled molecular system. A genetic algorithm and a new mid-IR polarization shaper were used to alter the relative vibrational excitation of the two carbonyl st...

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Bibliografische gegevens
Hoofdauteurs: Strasfeld, David B, Middleton, Chris T, Zanni, Martin T
Formaat: Artigo
Taal:Inglês
Gepubliceerd in: 2009
Onderwerpen:
Online toegang:https://ncbi.nlm.nih.gov/pmc/articles/PMC2867476/
https://ncbi.nlm.nih.gov/pubmed/20463848
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1088/1367-2630/11/10/105046
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